As far as I can tell, you cannot decrypt any of the assets that are already encrypted because of the fact that the assets may be tied to a session id. (They have different encrypted data for the same exact file, but different session. I may be wrong, the __info file may be tied to it.)
The only way forward is to have some sort of mod that prevents vrchat from encrypting the cache, BUT you have to bypass any security features to keep from being detected.
I suspect that vrchat is utilizing session based encryption and using something in the __info file to encrypt it as there is a large numerical number that changes each download.